受珊瑚启发的多尺度多孔颗粒嵌套结构,实现高效彩色辐射冷却
Coral‐Inspired Multi‐Scale Porous Particle‐Nested Structure for Efficient Colored Radiative Cooling
中文简介
被动白天辐射冷却(PDRC)是实现碳中和节能甚至减碳的最有前景方法之一。然而,开发既能有效冷却性能又符合户外美学要求的彩色 PDRC 材料仍具挑战。具有轻质、低成本且普遍高热发射率的高分子材料,具有高效辐射冷却材料的巨大潜力。本研究在聚合物框架中设计了层级孔-颗粒-嵌套结构,实现 93.6%的太阳反射率和 91.1%的热辐射率。此外,彩色变体保持了高性能,蓝色、粉色和黄色薄膜的太阳反射率分别为 80.6%、84.8%和 88.1%。孔隙-颗粒-嵌套结构增强了直射和漫射阳光的散射,使高效彩色 PDRC 薄膜得以实现。凭借更强的机械性能和疏水性能,该结构为开发实用的户外 PDRC 材料提供了一种经济高效的策略。
英文摘要(原文)
Passive daytime radiative cooling (PDRC) is one of the most promising ways for energy conservation and even carbon emission reduction to achieve carbon neutrality. However, developing colored PDRC materials that exhibit effective cooling performance while meeting aesthetic requirements for outdoor applications remains challenging. Polymer material with lightweight, low-cost, and universal high thermal emissivity, poses great potential of efficient radiative cooling materials. In this study, a hierarchical pore-particle-nested structure is engineered in a polymer framework, achieving a solar reflectance of 93.6% and a thermal emissivity of 91.1%. Moreover, the colored variants maintained high performance, with solar reflectance values of 80.6%, 84.8%, and 88.1% for the blue, pink, and yellow films, respectively. The pore-particle-nested structure enhances scattering of both direct and diffuse sunlight, enabling efficient colored PDRC films. With enhanced mechanical properties and hydrophobic performance, the structure provides a cost-effective strategy for developing practical outdoor PDRC materials.
题录(GB/T 7714)
Zhang Z, Song Z, Lu W, 等. Coral‐Inspired Multi‐Scale Porous Particle‐Nested Structure for Efficient Colored Radiative Cooling[J]. Small Methods, 2025, 10(3): e01374. DOI: 10.1002/smtd.202501374.
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